Quasi-particle Dynamics of a Strongly Correlated Polaron Metal

نویسندگان

  • J Zhong
  • H.-B Schüttler
چکیده

We develop a simple diagrammatic low-energy boson exchange strong-coupling model for an antiferromagnetically correlated polaronic metal. The model is based on a simplified, local anharmonic oscillator representation of the highly anharmonic Born-Oppenheimer lattice potential which typically arises in a finite density po-laron system, as a result of polaronic self-localization. This Born-Oppenheimer potential exhibits a large manifold of nearly degenrate local potential minima, and hence a new class of low-energy excitations, associated with tunneling processes between the multiple Born-Oppenheimer wells. In the present paper, we employ a simple Migdal-type single-exchange diagrammatic approximation in order to study the what happens when conduction electrons are coupled to these anharmonic tunneling excitations via conventional electron-phonon interactions. Important low-temperature features of such a model are (i) a large polaronic mass enhancement Z and a strongly narrowed, low-energy, near-Fermi-level van Hove resonance peak in the interacting density of states at temperatures T well below the lattice tunneling energy scale Ω t ; (ii) a rapid thermal suppression of Z and of the van Hove resonance which occurs when the temperature T becomes comparable to the lattice tunneling excitation energy scale Ω t ; (iii) a broad incoherent background in the single-particle spectra |G ′′ (k, ω)| near the Fermi energy; (iv) strongly flattened quasi-particle bands over wide regions of the Brillouin zone near the van Hove points; and (v) strong isotopic mass dependence of the elec-– 1 – tronic mass enhancement Z at temperatures T well below Ω t which, along with Z, becomes rapidly suppressed for T comparable to Ω t. Surprisingly, in spite of the large low-T mass enhancment, the anharmonic lattice fluctuations in the high temperature regime T > ∼ Ω t , give rise only to a moderate, essentially T-independent quasi-particle damping. This damping does not suppress coherent quasi-particle propagation in a wide, physically relevant parameter regime. We thus argue that, in a " weakly bound " finite-density polaron system, a novel polaron scenario may be realized where only the lattice motion, but not the quasi-particle propagation become incoherent in the high-T regime. This scenario is in contrast to the conventional small-polaron strong-coupling picture, where the quasi-particle transport inevitably becomes incoherent at temperatures exceeding the polaron tunneling energy scale. We also discuss possible implications of the anharmonic tunneling model for the cuprate superconductors. The predicted isotopic mass dependence of the low-T (T < Ω t) electron quasi-particle mass enhancement provides a unique …

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Localisation versus self-trapping: Polaron formation in the Anderson-Holstein model

The polaron concept, first introduced by Landau [1], is one of the main pillars on which the theoretical analysis of materials with strong electron-phonon (EP) coupling rests. In these compounds, the coupling between the electron and the lattice leads to a lattice deformation whose potential tends to bind the electron to the deformed region of the crystal. This process, which has been called se...

متن کامل

Localization properties of two interacting particles in a quasi-periodic potential with a metal-insulator transition

We study the influence of many-particle interactions on a metal-insulator transition. We consider the two-interacting-particle problem for onsite interacting particles on a one-dimensional quasiperiodic chain, the so-called Aubry-André model. We show numerically by the decimation method and finite-size scaling that the interaction does not modify the critical parameters such as the transition p...

متن کامل

Ultrafast Studies of Exciton Migration and Polaron Formation in Sequentially Solution-Processed Conjugated Polymer/Fullerene Quasi-Bilayer Photovoltaics.

We examine the ultrafast dynamics of exciton migration and polaron production in sequentially processed 'quasi-bilayer' and preblended 'bulk heterojunction' (BHJ) solar cells based on conjugated polymer films that contain the same total amount of fullerene. We find that even though the polaron yields are similar, the dynamics of polaron production are significantly slower in quasi-bilayers than...

متن کامل

Supplemental Material: “Polaron-to-polaron transitions in the radio-frequency spectrum of a quasi-two-dimensional Fermi gas”

In this supplemental material, we discuss the calculation of the radio-frequency spectra arising from confinement-induced dimers and polarons in a quasi-two-dimensional Fermi gas. We determine the dimer binding energies, including both the tight axial confinement and the nonzero transverse confinement. We provide the probabilities for dimer-to-dimer transitions and the shape of the dimerto-scat...

متن کامل

Influence of Interface Thermal Resistance on Relaxation Dynamics of Metal-Dielectric Nanocomposite Materials under Ultrafast Pulse Laser Excitation

Nanocomposite materials, including noble metal nanoparticles embedded in a dielectric host medium, are interesting because of their optical properties linked to surface plasmon resonance phenomena. For studding of nonlinear optical properties and/or energy transfer process, these materials may be excited by ultrashort pulse laser with a temporal width varying from some femtoseconds to some hund...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 1998